Super-resolution Control of Two-dimensional Quantum Emitters

Localized interlayer excitons in semiconducting transition-metal dichalcogenide heterobilayers are quantum emitters with a static electric dipole moment, making them excellent nanoscale charge sensors to probe correlated quantum phases in a proximal layer. These emitters are electrically tunable and inherit spin-valley selection rules, yet their deterministic spatial control remains challenging due to subwavelength confinement. Here, we present a platform that combines cryogenic optical spectroscopy with scanning probe microscopy to investigate trapped interlayer excitons in WSe$_2$/MoSe$_2$ bilayers. By exploiting AFM-based local Stark shift, we achieve super-resolution localization of emitters separated by only a few tens of nanometers and demonstrate deterministic control of individual charge states, including trion formation, opening a path towards coherent inter-dot coupling. Time-resolved measurements reveal tip-induced modification of the electromagnetic vacuum around individual emitters, thus controlling their radiative emission. Our multi-point charge sensing platform with optical readout is particularly well-suited to study fractionalization and anyon dynamics in semiconducting FCIs.